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If you put enough aerosol particulates in the stratosphere at 20 Km, you can reflect about 2-4 W/sq. meter of sunlight (shortwave IR radiation) back into space before it hits the Earth's surface and becomes blackbody long wave IR radiation which is readily absorbed by CO2, raising the temperature of the Earth to rebalance the energy equation, (ie., solar radiation energy in = blackbody radiation energy out). This form of geo-engineering is called Solar Radiation Mgt. or Stratospheric Aerosol Injection. The particulates chosen just have to have a high albedo at 0.2-5 microns wavelength. SO2 (sulfate) works, but so does CaCO3 (calcite) and some silicates (glass). The issue is that you need a lot of stuff high enough in the atmosphere so that it doesn't rain out in a couple days. If you eject it from an aircraft at 20 Km (65,000 ft.) it will stay up for 18 months. If you eject it in the Troposphere (<11 Km), where most commercial aircraft fly, it will dissipate in about a day. If you can get about 2-5 million tons of the stuff up, you can completely reverse ~ 2 degrees C of global warming.....at least until we figure out how to stop putting so much CO2 into the atmosphere. My role is to design a new aircraft big enough and with enough performance to carry 30,000 pounds of aerosol to 65,000 ft. Not so easy - the U-2S can get there, but can only carry about 1,000 pounds. Nothing else even comes close. Here's a pic of our aircraft - 172 ft. span, six GE F118 engines and a big tank of dust it is belly !
If you put enough aerosol particulates in the stratosphere at 20 Km, you can reflect about 2-4 W/sq. meter of sunlight (shortwave IR radiation) back into space before it hits the Earth's surface and becomes blackbody long wave IR radiation which is readily absorbed by CO2, raising the temperature of the Earth to rebalance the energy equation, (ie., solar radiation energy in = blackbody radiation energy out). This form of geo-engineering is called Solar Radiation Mgt. or Stratospheric Aerosol Injection. The particulates chosen just have to have a high albedo at 0.2-5 microns wavelength. SO2 (sulfate) works, but so does CaCO3 (calcite) and some silicates (glass). The issue is that you need a lot of stuff high enough in the atmosphere so that it doesn't rain out in a couple days. If you eject it from an aircraft at 20 Km (65,000 ft.) it will stay up for 18 months. If you eject it in the Troposphere (<11 Km), where most commercial aircraft fly, it will dissipate in about a day. If you can get about 2-5 million tons of the stuff up, you can completely reverse ~ 2 degrees C of global warming.....at least until we figure out how to stop putting so much CO2 into the atmosphere. My role is to design a new aircraft big enough and with enough performance to carry 30,000 pounds of aerosol to 65,000 ft. Not so easy - the U-2S can get there, but can only carry about 1,000 pounds. Nothing else even comes close.
Your proposal is intriguing, but also the stuff of cheap sci-fi nightmares. Hopefully it does fall out of the atmosphere and so doesn't make permanent change in case for some unforeseen reason we want warmer climate down the road. Fixing one technology based problem with another rarely seems to work. Plus sounds like it'll cut into my PV solar production.