The original tweeter was Eminence ASD:1001

The replacement tweeter is Radian 475PB

Main reasons it sounds bad: the two compression drivers have very different frequency response curve shapes, and they have very different sensitivity. The crossover is valid only for the Eminence driver. It will flatten out the bumpy response and match the level to the woofer. The unchanged crossover driving the Radian will play at least 6dB (2x) louder overall, and will be especially loud near 1kHz where Radian is 18dB louder than Eminence. That's what sounds like crap.
Your 2 possible solutions:
Replace the radian with new eminence drivers (matched from Zu) to restore factory performance.
Change the crossover to accommodate the Radian driver.
If Zu does use Radian drivers, then maybe they already have a crossover for 475PB with the FRD. You could contact them about buying those crossovers, talking about the feasibility of it. See whether the Radian actually works inside their Eminence-optimized waveguide.
You mention the Radian 850PB, but that is 2" throat diameter so it is totally incompatible with this speaker which has a 1" throat diameter waveguide. I doubt Zu would sell you the 2" waveguide without the rest of the speaker.
fwiw, having done a lot of DIY and mods, I'm of the mind now that modding is rarely the best path forward. My advice is to repair the Zus as stock, sell them and upgrade to the Zu Soul Supreme or whatever speakers that have the higher performance that you want.