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Constrained Damping Layer (CLD) works best when both panels are the same. That is, a CLD of 1/2 inch wallboard - Green Glue - 1/2 inch wallboard, will be better than a CLD of 5/8 inch wallboard - Green Glue - 1/2 inch wallboard.
While it is "Green" in color it is not a "Glue" in any sense.It has no adhesive properties.
Haha, I'm guessing you've never used it. Green Glue definately sticks two flat panels together very well and for a long time. Since it never hardens, the two panels aren't rigidly coupled, but that's a benefit in a case like this.